Perovskite phase stabilization in epitaxial Pb(Mg1/3Nb2/3)O3–PbTiO3Pb(Mg1/3Nb2/3)O3–PbTiO3 films by deposition onto vicinal (001) SrTiO3SrTiO3 substrates
dc.contributor.author | Bu, S. D. | en_US |
dc.contributor.author | Lee, M. K. | en_US |
dc.contributor.author | Eom, Chang-Beom | en_US |
dc.contributor.author | Tian, Wei | en_US |
dc.contributor.author | Pan, Xiaoqing | en_US |
dc.contributor.author | Streiffer, S. K. | en_US |
dc.contributor.author | Krajewski, J. J. | en_US |
dc.date.accessioned | 2010-05-06T21:52:42Z | |
dc.date.available | 2010-05-06T21:52:42Z | |
dc.date.issued | 2001-11-19 | en_US |
dc.identifier.citation | Bu, S. D.; Lee, M. K.; Eom, C. B.; Tian, W.; Pan, X. Q.; Streiffer, S. K.; Krajewski, J. J. (2001). "Perovskite phase stabilization in epitaxial Pb(Mg1/3Nb2/3)O3–PbTiO3Pb(Mg1/3Nb2/3)O3–PbTiO3 films by deposition onto vicinal (001) SrTiO3SrTiO3 substrates." Applied Physics Letters 79(21): 3482-3484. <http://hdl.handle.net/2027.42/70257> | en_US |
dc.identifier.uri | https://hdl.handle.net/2027.42/70257 | |
dc.description.abstract | We report the perovskite phase stabilization of 0.67Pb(Mg1/3Nb2/3)O3–0.33PbTiO30.67Pb(Mg1/3Nb2/3)O3–0.33PbTiO3 (PMN-PT) epitaxial thin films by deposition onto miscut substrates. Films were grown on (001) SrTiO3SrTiO3 substrates with miscut angles from 0 to 8 degrees toward the [100] direction using 90° off-axis magnetron sputtering. Films on high miscut substrates (>4°) showed almost the pure perovskite phase in both x-ray diffraction and transmission electron microscopy image, and were nearly stoichiometric. In contrast, films on exact (001) SrTiO3SrTiO3 contained a high volume fraction of pyrochlore phases with Pb deficiency. Atomic force microscopy reveals that films on 8° miscut substrates have a much smoother surface morphology than those on exact (001) SrTiO3.SrTiO3. Cross-sectional transmission electron microscopy images reveal that the pyrochlore phases nucleate on top of the perovskite phase, and that the amount of the pyrochlore phases increase with film thickness. A film on an 8° miscut substrate exhibits a polarization hysteresis loop with a remnent polarization of 20 μC/cm2μC/cm2 at room temperature. © 2001 American Institute of Physics. | en_US |
dc.format.extent | 3102 bytes | |
dc.format.extent | 197251 bytes | |
dc.format.mimetype | text/plain | |
dc.format.mimetype | application/pdf | |
dc.publisher | The American Institute of Physics | en_US |
dc.rights | © The American Institute of Physics | en_US |
dc.title | Perovskite phase stabilization in epitaxial Pb(Mg1/3Nb2/3)O3–PbTiO3Pb(Mg1/3Nb2/3)O3–PbTiO3 films by deposition onto vicinal (001) SrTiO3SrTiO3 substrates | en_US |
dc.type | Article | en_US |
dc.subject.hlbsecondlevel | Physics | en_US |
dc.subject.hlbtoplevel | Science | en_US |
dc.description.peerreviewed | Peer Reviewed | en_US |
dc.contributor.affiliationum | Department of Materials Science and Engineering, The University of Michigan, Ann Arbor, Michigan 48109 | en_US |
dc.contributor.affiliationother | Department of Materials Science and Engineering, University of Wisconsin-Madison, Madison, Wisconsin 53706 | en_US |
dc.contributor.affiliationother | Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 | en_US |
dc.contributor.affiliationother | Bell Laboratory, Lucent Technologies, Murray Hill, New Jersey 07974 | en_US |
dc.description.bitstreamurl | http://deepblue.lib.umich.edu/bitstream/2027.42/70257/2/APPLAB-79-21-3482-1.pdf | |
dc.identifier.doi | 10.1063/1.1414293 | en_US |
dc.identifier.source | Applied Physics Letters | en_US |
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