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Dynamic behavior of the monomer–monomer surface reaction model with adsorbate interactions

dc.contributor.authorVoigt, Christopher A.en_US
dc.contributor.authorZiff, Robert M.en_US
dc.date.accessioned2010-05-06T22:33:45Z
dc.date.available2010-05-06T22:33:45Z
dc.date.issued1997-11-08en_US
dc.identifier.citationVoigt, Christopher A.; Ziff, Robert M. (1997). "Dynamic behavior of the monomer–monomer surface reaction model with adsorbate interactions." The Journal of Chemical Physics 107(18): 7397-7401. <http://hdl.handle.net/2027.42/70692>en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/70692
dc.description.abstractThe monomer–monomer surface reaction model with an adsorbate interaction term is studied. An epidemic analysis of the poisoning times (tp)(tp) for small square lattices as a function of lattice edge length LL and interaction strength α at the point of equal adsorption rates yields a dynamic scaling relation which describes the crossover between log-power-law and exponential behavior in L,L, and is able to fit the entire dependence of tptp upon α and L.L. The phase transition is further explored by varying adsorption rates and is found to follow second-order kinetics. A mean-field approximation is introduced as a comparison for the numerical results. © 1997 American Institute of Physics.en_US
dc.format.extent3102 bytes
dc.format.extent134479 bytes
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dc.format.mimetypeapplication/pdf
dc.publisherThe American Institute of Physicsen_US
dc.rights© The American Institute of Physicsen_US
dc.titleDynamic behavior of the monomer–monomer surface reaction model with adsorbate interactionsen_US
dc.typeArticleen_US
dc.subject.hlbsecondlevelPhysicsen_US
dc.subject.hlbtoplevelScienceen_US
dc.description.peerreviewedPeer Revieweden_US
dc.contributor.affiliationumDepartment of Chemical Engineering, University of Michigan, Ann Arbor, Michigan 48109-2136en_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/70692/2/JCPSA6-107-18-7397-1.pdf
dc.identifier.doi10.1063/1.474977en_US
dc.identifier.sourceThe Journal of Chemical Physicsen_US
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dc.owningcollnamePhysics, Department of


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