Phase-matched optical parametric conversion of ultrashort pulses in a hollow waveguide

Abstract

We demonstrate for the first time nonresonant phase-matched frequency conversion of ultrashort pulses in gases. Broad-bandwidth ultrafast pulses, tunable around 270 nm, were generated from a Ti:sapphire amplifier system using 2ω+2ω−ω2ω+2ω−ω parametric wave mixing in a capillary waveguide. Both the fundamental and the second-harmonic light were coupled into the lowest-order (EH11)(EH11) mode. The output pulses have an energy >4μJ at a 1kHz repetition rate, in the EH11EH11 spatial mode. This method can be made to generate 10–20fs pulses, and is the first phase-matching technique which is applicable to frequency conversion into the deep- and vacuum-ultraviolet regions of the spectrum. © 1998 American Institute of Physics.