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Reconciling modeled and observed atmospheric deposition of soluble organic nitrogen at coastal locations
dc.contributor.authorIto, Akinorien_US
dc.contributor.authorLin, Guangxingen_US
dc.contributor.authorPenner, Joyce E.en_US
dc.date.accessioned2014-08-06T16:49:45Z
dc.date.availableWITHHELD_11_MONTHSen_US
dc.date.available2014-08-06T16:49:45Z
dc.date.issued2014-06en_US
dc.identifier.citationIto, Akinori; Lin, Guangxing; Penner, Joyce E. (2014). "Reconciling modeled and observed atmospheric deposition of soluble organic nitrogen at coastal locations." Global Biogeochemical Cycles 28(6): 617-630.en_US
dc.identifier.issn0886-6236en_US
dc.identifier.issn1944-9224en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/108038
dc.description.abstractAtmospheric deposition of reactive nitrogen (N) species from air pollutants is a significant source of exogenous nitrogen in marine ecosystems. Here we use an atmospheric chemical transport model to investigate the supply of soluble organic nitrogen (ON) from anthropogenic sources to the ocean. Comparisons of modeled deposition with observations at coastal and marine locations show good overall agreement for inorganic nitrogen and total soluble nitrogen. However, previous modeling approaches result in significant underestimates of the soluble ON deposition if the model only includes the primary soluble ON and the secondary oxidized ON in gases and aerosols. Our model results suggest that including the secondary reduced ON in aerosols as a source of soluble ON contributes to an improved prediction of the deposition rates (g N m −2  yr −1 ). The model results show a clear distinction in the vertical distribution of soluble ON in aerosols between different processes from the primary sources and the secondary formation. The model results (excluding the biomass burning and natural emission changes) suggest an increase in soluble ON outflow from atmospheric pollution, in particular from East Asia, to the oceans in the twentieth century. These results highlight the necessity of improving the process‐based quantitative understanding of the chemical reactions of inorganic nitrogen species with organics in aerosol and cloud water. Key Points Soluble secondary reduced ON improves model‐observation comparison Vertical profile of soluble ON differs between different formation processes Human activities increase terrestrial soluble ON input to the oceansen_US
dc.publisherWiley Periodicals, Inc.en_US
dc.subject.otherOrganic Nitrogenen_US
dc.subject.otherOxidized Nitrogenen_US
dc.subject.otherReduced Nitrogenen_US
dc.subject.otherEnvironmental Changesen_US
dc.subject.otherAtmospheric Depositionen_US
dc.titleReconciling modeled and observed atmospheric deposition of soluble organic nitrogen at coastal locationsen_US
dc.typeArticleen_US
dc.rights.robotsIndexNoFollowen_US
dc.subject.hlbsecondlevelGeological Sciencesen_US
dc.subject.hlbtoplevelScienceen_US
dc.description.peerreviewedPeer Revieweden_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/108038/1/TableS2.pdf
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/108038/2/TableS1.pdf
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/108038/3/GBC_02042013readme.pdf
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/108038/4/gbc20169.pdf
dc.identifier.doi10.1002/2013GB004721en_US
dc.identifier.sourceGlobal Biogeochemical Cyclesen_US
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