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Radiative forcing of organic aerosol in the atmosphere and on snow: Effects of SOA and brown carbon
dc.contributor.authorLin, Guangxingen_US
dc.contributor.authorPenner, Joyce E.en_US
dc.contributor.authorFlanner, Mark G.en_US
dc.contributor.authorSillman, Sanforden_US
dc.contributor.authorXu, Lien_US
dc.contributor.authorZhou, Chengen_US
dc.date.accessioned2014-08-06T16:49:53Z
dc.date.availableWITHHELD_11_MONTHSen_US
dc.date.available2014-08-06T16:49:53Z
dc.date.issued2014-06-27en_US
dc.identifier.citationLin, Guangxing; Penner, Joyce E.; Flanner, Mark G.; Sillman, Sanford; Xu, Li; Zhou, Cheng (2014). "Radiative forcing of organic aerosol in the atmosphere and on snow: Effects of SOA and brown carbon." Journal of Geophysical Research: Atmospheres 119(12): 7453-7476.en_US
dc.identifier.issn2169-897Xen_US
dc.identifier.issn2169-8996en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/108060
dc.description.abstractOrganic aerosols (OA) play an important role in climate change. However, very few calculations of global OA radiative forcing include secondary organic aerosol (SOA) or the light‐absorbing part of OA (brown carbon). Here we use a global model to assess the radiative forcing associated with the change in primary organic aerosol (POA) and SOA between present‐day and preindustrial conditions in both the atmosphere and the land snow/sea ice. Anthropogenic emissions are shown to substantially influence the SOA formation rate, causing it to increase by 29 Tg/yr (93%) since preindustrial times. We examine the effects of varying the refractive indices, size distributions for POA and SOA, and brown carbon fraction in SOA. The increase of SOA exerts a direct forcing ranging from −0.12 to −0.31 W m −2 and a first indirect forcing in warm‐phase clouds ranging from −0.22 to −0.29 W m −2 , with the range due to different assumed SOA size distributions and refractive indices. The increase of POA since preindustrial times causes a direct forcing varying from −0.06 to −0.11 W m −2 , when strongly and weakly absorbing refractive indices for brown carbon are used. The change in the total OA exerts a direct forcing ranging from −0.14 to −0.40 W m −2 . The atmospheric absorption from brown carbon ranges from +0.22 to +0.57 W m −2 , which corresponds to 27%~70% of the black carbon (BC) absorption predicted in the model. The radiative forcing of OA deposited in land snow and sea ice ranges from +0.0011 to +0.0031 W m −2 or as large as 24% of the forcing caused by BC in snow and ice simulated by the model. Key Points A fully explicit SOA formation model is used to determine SOA radiative forcing The direct radiative forcing by brown carbon in SOA is estimated The radiative forcing of OA in snow/ice is estimated for the first timeen_US
dc.publisherWiley Periodicals, Inc.en_US
dc.publisherCambridge Univ. Pressen_US
dc.subject.otherOrganic Aerosolen_US
dc.subject.otherSOAen_US
dc.subject.otherRadiative Forcingen_US
dc.subject.otherBrown Carbonen_US
dc.subject.otherClimate Changeen_US
dc.subject.otherAtmospheric Chemistryen_US
dc.titleRadiative forcing of organic aerosol in the atmosphere and on snow: Effects of SOA and brown carbonen_US
dc.typeArticleen_US
dc.rights.robotsIndexNoFollowen_US
dc.subject.hlbsecondlevelAtmospheric and Oceanic Sciencesen_US
dc.subject.hlbtoplevelScienceen_US
dc.description.peerreviewedPeer Revieweden_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/108060/1/jgrd51450.pdf
dc.identifier.doi10.1002/2013JD021186en_US
dc.identifier.sourceJournal of Geophysical Research: Atmospheresen_US
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dc.owningcollnameInterdisciplinary and Peer-Reviewed


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