Towards a Safe Lithium–Sulfur Battery with a Flame‐Inhibiting Electrolyte and a Sulfur‐Based Composite Cathode
dc.contributor.author | Wang, Jiulin | en_US |
dc.contributor.author | Lin, Fengjiao | en_US |
dc.contributor.author | Jia, Hao | en_US |
dc.contributor.author | Yang, Jun | en_US |
dc.contributor.author | Monroe, Charles W. | en_US |
dc.contributor.author | NuLi, Yanna | en_US |
dc.date.accessioned | 2014-10-07T16:09:33Z | |
dc.date.available | WITHHELD_12_MONTHS | en_US |
dc.date.available | 2014-10-07T16:09:33Z | |
dc.date.issued | 2014-09-15 | en_US |
dc.identifier.citation | Wang, Jiulin; Lin, Fengjiao; Jia, Hao; Yang, Jun; Monroe, Charles W.; NuLi, Yanna (2014). "Towards a Safe Lithium–Sulfur Battery with a Flame‐Inhibiting Electrolyte and a Sulfur‐Based Composite Cathode ." Angewandte Chemie 126(38): 10263-10268. | en_US |
dc.identifier.issn | 0044-8249 | en_US |
dc.identifier.issn | 1521-3757 | en_US |
dc.identifier.uri | https://hdl.handle.net/2027.42/108645 | |
dc.description.abstract | Of the various beyond‐lithium‐ion batteries, lithium–sulfur (Li‐S) batteries were recently reported as possibly being the closest to market. However, its theoretically high energy density makes it potentially hazardous under conditions of abuse. Therefore, addressing the safety issues of Li‐S cells is necessary before they can be used in practical applications. Here, we report a concept to build a safe and highly efficient Li‐S battery with a flame‐inhibiting electrolyte and a sulfur‐based composite cathode. The flame retardant not only makes the carbonates nonflammable but also dramatically enhances the electrochemical performance of the sulfur‐based composite cathode, without an apparent capacity decline over 750 cycles, and with a capacity greater than 800 mA h −1 g −1 (sulfur) at a rate of 10 C. Feuertaufe : Eine nichtentzündbare Schwefelkompositkathode zeigt eine stabile elektrochemische Aktivität über 750 Zyklen und eine Entladungskapazität von über 800 mA h −1 g −1 (Schwefel) mit einer Entladerate von 10 C in einem feuersicheren Elektrolyten. Der Elektrolyt wurde aus einem Phosphitadditiv erzeugt, das an Grenzflächenreaktionen an der Kathode teilnimmt und die Lithiumionendiffusion um das mehr als Zehnfache beschleunigt. | en_US |
dc.publisher | WILEY‐VCH Verlag | en_US |
dc.subject.other | Feuersichere Elektrolyte | en_US |
dc.subject.other | Lithium | en_US |
dc.subject.other | Schwefel | en_US |
dc.subject.other | Elektrochemie | en_US |
dc.subject.other | Batterien | en_US |
dc.title | Towards a Safe Lithium–Sulfur Battery with a Flame‐Inhibiting Electrolyte and a Sulfur‐Based Composite Cathode | en_US |
dc.type | Article | en_US |
dc.rights.robots | IndexNoFollow | en_US |
dc.subject.hlbsecondlevel | Chemical Engineering | en_US |
dc.subject.hlbsecondlevel | Chemistry | en_US |
dc.subject.hlbsecondlevel | Materials Science and Engineering | en_US |
dc.subject.hlbtoplevel | Engineering | en_US |
dc.subject.hlbtoplevel | Science | en_US |
dc.description.peerreviewed | Peer Reviewed | en_US |
dc.contributor.affiliationum | Department of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109 (USA) | en_US |
dc.contributor.affiliationother | School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240 (China) | en_US |
dc.description.bitstreamurl | http://deepblue.lib.umich.edu/bitstream/2027.42/108645/1/ange_201405157_sm_miscellaneous_information.pdf | |
dc.description.bitstreamurl | http://deepblue.lib.umich.edu/bitstream/2027.42/108645/2/10263_ftp.pdf | |
dc.identifier.doi | 10.1002/ange.201405157 | en_US |
dc.identifier.source | Angewandte Chemie | en_US |
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