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Homogeneous and Heterogeneous Photocatalytic Water Oxidation by Persulfate
dc.contributor.authorFukuzumi, Shunichi
dc.contributor.authorJung, Jieun
dc.contributor.authorYamada, Yusuke
dc.contributor.authorKojima, Takahiko
dc.contributor.authorNam, Wonwoo
dc.date.accessioned2017-06-16T20:07:57Z
dc.date.available2017-06-16T20:07:57Z
dc.date.issued2016-04-20
dc.identifier.citationFukuzumi, Shunichi; Jung, Jieun; Yamada, Yusuke; Kojima, Takahiko; Nam, Wonwoo (2016). "Homogeneous and Heterogeneous Photocatalytic Water Oxidation by Persulfate." Chemistry – An Asian Journal 11(8): 1138-1150.
dc.identifier.issn1861-4728
dc.identifier.issn1861-471X
dc.identifier.urihttps://hdl.handle.net/2027.42/137224
dc.description.abstractPhotocatalytic water oxidation by persulfate (Na2S2O8) with [Ru(bpy)3]2+ (bpy=2,2′‐bipyridine) as a photocatalyst provides a standard protocol to study the catalytic reactivity of water oxidation catalysts. The yield of evolved oxygen per persulfate is regarded as a good index for the catalytic reactivity because the oxidation of bpy of [Ru(bpy)3]2+ and organic ligands of catalysts competes with the catalytic water oxidation. A variety of metal complexes act as catalysts in the photocatalytic water oxidation by persulfate with [Ru(bpy)3]2+ as a photocatalyst. Herein, the catalytic mechanisms are discussed for homogeneous water oxidation catalysis. Some metal complexes are converted to metal oxide or hydroxide nanoparticles during the photocatalytic water oxidation by persulfate, acting as precursors for the actual catalysts. The catalytic reactivity of various metal oxides is compared based on the yield of evolved oxygen and turnover frequency. A heteropolynuclear cyanide complex is the best catalyst reported so far for the photocatalytic water oxidation by persulfate and [Ru(bpy)3]2+, affording 100 % yield of O2 per persulfate.Waterworld: Homogeneous and heterogeneous catalysis and mechanisms of photocatalytic oxidation of water by persulfate with [Ru(bpy)]32+ are compared and discussed including the conversion from homogeneous precatalysts to heterogeneous catalysts.
dc.publisherWiley Periodicals, Inc.
dc.subject.otherhomogeneous catalysis
dc.subject.otherheterogeneous catalysis
dc.subject.othernanoparticles
dc.subject.otherphotocatalysis
dc.subject.otherwater oxidation
dc.titleHomogeneous and Heterogeneous Photocatalytic Water Oxidation by Persulfate
dc.typeArticleen_US
dc.rights.robotsIndexNoFollow
dc.subject.hlbsecondlevelChemistry
dc.subject.hlbtoplevelScience
dc.description.peerreviewedPeer Reviewed
dc.description.bitstreamurlhttps://deepblue.lib.umich.edu/bitstream/2027.42/137224/1/asia201501329.pdf
dc.description.bitstreamurlhttps://deepblue.lib.umich.edu/bitstream/2027.42/137224/2/asia201501329_am.pdf
dc.identifier.doi10.1002/asia.201501329
dc.identifier.sourceChemistry – An Asian Journal
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dc.owningcollnameInterdisciplinary and Peer-Reviewed


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