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Efficient Photocatalytic Water Reduction Using Inâ Situ Generated Knölker’s Iron Complexes
dc.contributor.authorSun, Yuan‐yuan
dc.contributor.authorWang, Hai
dc.contributor.authorChen, Nan‐yu
dc.contributor.authorLennox, Alastair J J
dc.contributor.authorFriedrich, Aleksej
dc.contributor.authorXia, Liang‐min
dc.contributor.authorLochbrunner, Stefan
dc.contributor.authorJunge, Henrik
dc.contributor.authorBeller, Matthias
dc.contributor.authorZhou, Shaolin
dc.contributor.authorLuo, Shu‐ping
dc.date.accessioned2017-06-16T20:10:57Z
dc.date.available2017-09-06T14:20:20Zen
dc.date.issued2016-07-20
dc.identifier.citationSun, Yuan‐yuan ; Wang, Hai; Chen, Nan‐yu ; Lennox, Alastair J J; Friedrich, Aleksej; Xia, Liang‐min ; Lochbrunner, Stefan; Junge, Henrik; Beller, Matthias; Zhou, Shaolin; Luo, Shu‐ping (2016). "Efficient Photocatalytic Water Reduction Using Inâ Situ Generated Knölker’s Iron Complexes." ChemCatChem 8(14): 2340-2344.
dc.identifier.issn1867-3880
dc.identifier.issn1867-3899
dc.identifier.urihttps://hdl.handle.net/2027.42/137356
dc.description.abstractInâ situ generated ironâ based Knölker complexes were found to be efficient catalysts in a fully nonâ noble metal Cuâ Fe photocatalytic water reduction system. These mononuclear iron catalysts were able to generate hydrogen up to 15 times faster than previously reported [Fe3(CO)12]. A reductive quenching mechanism was shown to operate by fluorescence experiments.Photo finish: Inâ situ generated ironâ based Knölker complexes are efficient catalysts in a fully nonâ noble metal Cuâ Fe photocatalytic water reduction system. These mononuclear iron catalysts generate hydrogen up to 15 times faster than previously reported [Fe3(CO)12]. A reductive quenching mechanism is shown to operate by fluorescence experiments. CuPS=copper(I) photosensitizer; SR=sacrificial reductant.
dc.publisherWiley Periodicals, Inc.
dc.subject.otherhydrogen
dc.subject.otherphotocatalysis
dc.subject.otherreduction
dc.subject.otherwater splitting
dc.subject.otheriron
dc.titleEfficient Photocatalytic Water Reduction Using Inâ Situ Generated Knölker’s Iron Complexes
dc.typeArticleen_US
dc.rights.robotsIndexNoFollow
dc.subject.hlbsecondlevelChemistry
dc.subject.hlbtoplevelScience
dc.description.peerreviewedPeer Reviewed
dc.description.bitstreamurlhttps://deepblue.lib.umich.edu/bitstream/2027.42/137356/1/cctc201600186.pdf
dc.description.bitstreamurlhttps://deepblue.lib.umich.edu/bitstream/2027.42/137356/2/cctc201600186_am.pdf
dc.description.bitstreamurlhttps://deepblue.lib.umich.edu/bitstream/2027.42/137356/3/cctc201600186-sup-0001-misc_information.pdf
dc.identifier.doi10.1002/cctc.201600186
dc.identifier.sourceChemCatChem
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