Understanding Molecular Structures of Buried Interfaces in Halide Perovskite Photovoltaic Devices Nondestructively with Sub‐Monolayer Sensitivity Using Sum Frequency Generation Vibrational Spectroscopy
dc.contributor.author | Xiao, Minyu | |
dc.contributor.author | Lu, Tieyi | |
dc.contributor.author | Lin, Ting | |
dc.contributor.author | Andre, John S. | |
dc.contributor.author | Chen, Zhan | |
dc.date.accessioned | 2020-08-10T20:54:34Z | |
dc.date.available | WITHHELD_12_MONTHS | |
dc.date.available | 2020-08-10T20:54:34Z | |
dc.date.issued | 2020-07 | |
dc.identifier.citation | Xiao, Minyu; Lu, Tieyi; Lin, Ting; Andre, John S.; Chen, Zhan (2020). "Understanding Molecular Structures of Buried Interfaces in Halide Perovskite Photovoltaic Devices Nondestructively with Sub‐Monolayer Sensitivity Using Sum Frequency Generation Vibrational Spectroscopy." Advanced Energy Materials 10(26): n/a-n/a. | |
dc.identifier.issn | 1614-6832 | |
dc.identifier.issn | 1614-6840 | |
dc.identifier.uri | https://hdl.handle.net/2027.42/156190 | |
dc.description.abstract | As performance of halide perovskite devices progresses, the device structure becomes more complex with more layers. Molecular interfacial structures between different layers play an increasingly important role in determining the overall performance in a halide perovskite device. However, current understanding of such interfacial structures at a molecular level nondestructively is limited, partially due to a lack of appropriate analytical tools to probe buried interfacial molecular structures in situ. Here, sum frequency generation (SFG) vibrational spectroscopy, a state‐of‐the‐art nonlinear interface sensitive spectroscopy, is introduced to the halide perovskite research community and is presented as a powerful tool to understand molecule behavior at buried halide perovskite interfaces in situ. It is found that interfacial molecular orientations revealed by SFG can be directly correlated to halide perovskite device performance. Here how SFG can examine molecular structures (e.g., orientations) at the perovskite/hole transporting layer and perovskite/electron transporting layer interfaces is discussed. This will promote the use of SFG to investigate molecular structures of buried interfaces in various halide perovskite materials and devices in situ nondestructively with a sub‐monolayer interface sensitivity. Such research will help to elucidate structure–function relationships of buried interfaces, aiding in the rational design/development of halide perovskite materials/devices with improved performance.Sum frequency generation vibrational spectroscopy, a state‐of‐the‐art nonlinear vibrational spectroscopy, is applied to elucidate molecular structure at buried halide perovskite interfaces in situ nondestructively with sub‐monolayer sensitivity. Molecular interfacial structures between different layers play an increasingly important, sometimes vital role in determining the overall performance in a halide perovskite device. | |
dc.publisher | Wiley Periodicals, Inc. | |
dc.subject.other | sum frequency generation vibrational spectroscopy | |
dc.subject.other | buried interfaces | |
dc.subject.other | molecular structures | |
dc.subject.other | perovskite photovoltaics | |
dc.subject.other | semiconducting polymers | |
dc.title | Understanding Molecular Structures of Buried Interfaces in Halide Perovskite Photovoltaic Devices Nondestructively with Sub‐Monolayer Sensitivity Using Sum Frequency Generation Vibrational Spectroscopy | |
dc.type | Article | |
dc.rights.robots | IndexNoFollow | |
dc.subject.hlbsecondlevel | Materials Science and Engineering | |
dc.subject.hlbtoplevel | Engineering | |
dc.description.peerreviewed | Peer Reviewed | |
dc.description.bitstreamurl | http://deepblue.lib.umich.edu/bitstream/2027.42/156190/2/aenm201903053_am.pdf | en_US |
dc.description.bitstreamurl | http://deepblue.lib.umich.edu/bitstream/2027.42/156190/1/aenm201903053.pdf | en_US |
dc.identifier.doi | 10.1002/aenm.201903053 | |
dc.identifier.source | Advanced Energy Materials | |
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dc.owningcollname | Interdisciplinary and Peer-Reviewed |
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