View Item 

Show simple item record

Lower Energy Excitation of Water Soluble Near-Infrared Emitting Mixed-Ligand Metallacrowns
dc.contributor.authorNguyen, Tu N.
dc.contributor.authorEliseeva, Svetlana V.
dc.contributor.authorMartinić, Ivana
dc.contributor.authorCarver, Peggy L.
dc.contributor.authorLathion, Timothée
dc.contributor.authorPetoud, Stéphane
dc.contributor.authorPecoraro, Vincent L.
dc.date.accessioned2023-06-01T20:51:20Z
dc.date.available2024-06-01 16:51:18en
dc.date.available2023-06-01T20:51:20Z
dc.date.issued2023-05-22
dc.identifier.citationNguyen, Tu N.; Eliseeva, Svetlana V.; Martinić, Ivana ; Carver, Peggy L.; Lathion, Timothée ; Petoud, Stéphane ; Pecoraro, Vincent L. (2023). "Lower Energy Excitation of Water Soluble Near- Infrared Emitting Mixed- Ligand Metallacrowns." Chemistry - A European Journal 29(29): n/a-n/a.
dc.identifier.issn0947-6539
dc.identifier.issn1521-3765
dc.identifier.urihttps://hdl.handle.net/2027.42/176880
dc.description.abstractBy combining advantages of two series of lanthanide(III)/zinc(II) metallacrowns (MCs) assembled using pyrazine- (pyzHA2−) and quinoxaline- (quinoHA2−) hydroximate building blocks ligands, we created here water-soluble mixed-ligand MCs with extended absorption to the visible range. The YbIII analogue demonstrated improved photophysical properties in the near-infrared (NIR) range in cell culture media, facilitating its application for NIR optical imaging in living HeLa cells.The best of both worlds: Water solubility of Zn16Ln(pyzHA)16 (H2pyzHA: pyrazine hydroxamic acid) or lower energy excitation of Zn16Ln(quinoHA)16 (H2quinoHA: quinoxaline hydroxamic acid) metallacrowns (MCs)? No need to choose! In water soluble mixed-ligand Zn16Yb(pyzHA)x(quinoHA)16–x MCs characteristic emission of YbIII in the near-infrared range can be sensitized upon excitation up to 600 nm in the solid state or 500 nm in aqueous solution.
dc.publisherWiley Periodicals, Inc.
dc.publisherElsevier Science B. V.
dc.subject.otherlanthanide
dc.subject.otherluminescence
dc.subject.othermetallacrown
dc.subject.othernear-infrared
dc.subject.otheroptical imaging
dc.titleLower Energy Excitation of Water Soluble Near-Infrared Emitting Mixed-Ligand Metallacrowns
dc.typeArticle
dc.rights.robotsIndexNoFollow
dc.subject.hlbsecondlevelChemistry
dc.subject.hlbtoplevelScience
dc.description.peerreviewedPeer Reviewed
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/176880/1/chem202300226.pdf
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/176880/2/chem202300226_am.pdf
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/176880/3/chem202300226-sup-0001-misc_information.pdf
dc.identifier.doi10.1002/chem.202300226
dc.identifier.sourceChemistry – A European Journal
dc.identifier.citedreferenceJ.-Y. Hu, Y. Ning, Y.-S. Meng, J. Zhang, Z.-Y. Wu, S. Gao, J.-L. Zhang, Chem. Sci. 2017, 8, 2702 – 2709;
dc.identifier.citedreferenceY. Cai, Z. Wei, C. Song, C. Tang, W. Han, X. Dong, Chem. Soc. Rev. 2019, 48, 22 – 37;
dc.identifier.citedreferenceJ. Xu, A. Gulzar, P. Yang, H. Bi, D. Yang, S. Gai, F. He, J. Lin, B. Xing, D. Jin, Coord. Chem. Rev. 2019, 381, 104 – 134;
dc.identifier.citedreferenceY. Fan, F. Zhang, Adv. Opt. Mater. 2019, 7, 1801417;
dc.identifier.citedreferenceI. Martinić, S. V. Eliseeva, S. Petoud, J. Lumin. 2017, 189, 19 – 43.
dc.identifier.citedreference 
dc.identifier.citedreferenceY. Y. Ning, M. L. Zhu, J. L. Zhang, Coord. Chem. Rev. 2019, 399, 213028;
dc.identifier.citedreferenceG.-Q. Jin, Y. Ning, J.-X. Geng, Z.-F. Jiang, Y. Wang, J.-L. Zhang, Inorg. Chem. Front. 2020, 7, 289 – 299;
dc.identifier.citedreferenceJ.-C. G. Bünzli, Chem. Rev. 2010, 110, 2729 – 2755;
dc.identifier.citedreferenceS. V. Eliseeva, J.-C. G. Bünzli, Chem. Soc. Rev. 2010, 39, 189 – 227.
dc.identifier.citedreference 
dc.identifier.citedreferenceS. Comby, J.-C. G. Bünzli, in Handbook on the Physics and Chemistry of Rare Earths, Vol. 37, Ch. 235 (Eds.: K. A. Gschneidner Jr., J.-C. G. Bünzli, V. K. Pecharsky ), Elsevier Science B. V., Amsterdam, 2007, pp. 217 – 470;
dc.identifier.citedreferenceI. Hernández, W. P. Gillin, in Handbook on the Physics and Chemistry of Rare Earths, Vol. 47 (Eds.: J.-C. G. Bünzli, V. K. Pecharsky ), Elsevier, 2015, pp. 1 – 100;
dc.identifier.citedreferenceJ.-C. G. Bünzli, S. V. Eliseeva, in Comprehensive Inorganic Chemistry II, Vol. 8 (Ed.: V. W.-W. Yam ), Elsevier B. V., Amsterdam, 2013, pp. 339 – 398;
dc.identifier.citedreferenceG.-Q. Jin, C. V. Chau, J. F. Arambula, S. Gao, J. L. Sessler, J.-L. Zhang, Chem. Soc. Rev. 2022, 51, 6177 – 6209;
dc.identifier.citedreferenceY. Ning, J. Tang, Y.-W. Liu, J. Jing, Y. Sun, J.-L. Zhang, Chem. Sci. 2018, 9, 3742 – 3753;
dc.identifier.citedreferenceY. Ning, Y.-W. Liu, Z.-S. Yang, Y. Yao, L. Kang, J. L. Sessler, J.-L. Zhang, J. Am. Chem. Soc. 2020, 142, 6761 – 6768.
dc.identifier.citedreference 
dc.identifier.citedreferenceY. Hasegawa, Y. Kitagawa, T. Nakanishi, NPG Asia Mater. 2018, 10, 52 – 70;
dc.identifier.citedreferenceH. Uh, S. Petoud, C. R. Chim. 2010, 13, 668 – 680.
dc.identifier.citedreferenceJ. Jankolovits, C. M. Andolina, J. W. Kampf, K. N. Raymond, V. L. Pecoraro, Angew. Chem. Int. Ed. 2011, 50, 9660 – 9664; Angew. Chem. 2011, 123, 9834 – 9838.
dc.identifier.citedreferenceI. Martinić, S. V. Eliseeva, T. N. Nguyen, V. L. Pecoraro, S. Petoud, J. Am. Chem. Soc. 2017, 139, 8388 – 8391.
dc.identifier.citedreferenceE. R. Trivedi, S. V. Eliseeva, J. Jankolovits, M. M. Olmstead, S. Petoud, V. L. Pecoraro, J. Am. Chem. Soc. 2014, 136, 1526 – 1534.
dc.identifier.citedreferenceS. V. Eliseeva, T. N. Nguyen, J. W. Kampf, E. R. Trivedi, V. L. Pecoraro, S. Petoud, Chem. Sci. 2022, 13, 2919 – 2931.
dc.identifier.citedreferenceI. Martinić, S. V. Eliseeva, T. N. Nguyen, F. Foucher, D. Gosset, F. Westall, V. L. Pecoraro, S. Petoud, Chem. Sci. 2017, 8, 6042 – 6050.
dc.identifier.citedreference 
dc.identifier.citedreferenceH. Wei, Z. Zhao, C. Wei, G. Yu, Z. Liu, B. Zhang, J. Bian, Z. Bian, C. Huang, Adv. Funct. Mater. 2016, 26, 2085 – 2096;
dc.identifier.citedreferenceM. Ganapathi, S. V. Eliseeva, N. R. Brooks, D. Soccol, J. Fransaer, K. Binnemans, J. Mater. Chem. 2012, 22, 5514 – 5522.
dc.identifier.citedreference 
dc.identifier.citedreferenceB. R. Smith, S. S. Gambhir, Chem. Rev. 2017, 117, 901 – 986;
dc.identifier.citedreferenceS. He, J. Song, J. Qu, Z. Cheng, Chem. Soc. Rev. 2018, 47, 4258 – 4278;
dc.identifier.citedreferenceKenry, Y. Duan, B. Liu, Adv. Mater. 2018, 30, e1802394;
dc.identifier.citedreferenceQ. Miao, K. Pu, Adv. Mater. 2018, 30, e1801778;
dc.identifier.citedreferenceC. Wang, Z. Wang, T. Zhao, Y. Li, G. Huang, B. D. Sumer, J. Gao, Biomat. 2018, 157, 62 – 75.
dc.identifier.citedreferenceG. Chen, I. Roy, C. Yang, P. N. Prasad, Chem. Rev. 2016, 116, 2826 – 2885.
dc.identifier.citedreference 
dc.working.doiNOen
dc.owningcollnameInterdisciplinary and Peer-Reviewed


Files in this item

Name:
chem202300226.pdf
Size:
698.3KB
Format:
PDF
View/Open
Name:
chem202300226_am.pdf
Size:
1.001MB
Format:
PDF
View/Open
Name:
chem202300226-sup-0001-misc_in ...
Size:
990.8KB
Format:
PDF
View/Open

Show simple item record

Remediation of Harmful Language

The University of Michigan Library aims to describe library materials in a way that respects the people and communities who create, use, and are represented in our collections. Report harmful or offensive language in catalog records, finding aids, or elsewhere in our collections anonymously through our metadata feedback form. More information at Remediation of Harmful Language.

Accessibility

If you are unable to use this file in its current format, please select the Contact Us link and we can modify it to make it more accessible to you.