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Suppressed physical aging in PMMA-titanium oxide nanocomposites by controlling alignment of nanoparticles
dc.contributor.authorHuo, Miao
dc.contributor.authorMa, Mingchao
dc.contributor.authorTeng, Yinuo
dc.contributor.authorXiao, Yuhan
dc.contributor.authorGuo, Yunlong
dc.date.accessioned2023-07-14T13:54:53Z
dc.date.available2024-08-14 09:54:52en
dc.date.available2023-07-14T13:54:53Z
dc.date.issued2023-07-20
dc.identifier.citationHuo, Miao; Ma, Mingchao; Teng, Yinuo; Xiao, Yuhan; Guo, Yunlong (2023). "Suppressed physical aging in PMMA-titanium oxide nanocomposites by controlling alignment of nanoparticles." Journal of Applied Polymer Science 140(28): n/a-n/a.
dc.identifier.issn0021-8995
dc.identifier.issn1097-4628
dc.identifier.urihttps://hdl.handle.net/2027.42/177224
dc.description.abstractThis study investigates the physical aging process of PMMA-TiO2 nanocomposites with different particle alignments. By using an external electric field to control the alignment of TiO2 particles, a uniform distribution of TiO2 particles in PMMA is transformed into a micrometer-level pillar structure. The physical aging process is measured using differential scanning calorimetry, and the particle alignment is confirmed by microscopy. Comparison of the aging behavior of different samples shows that the addition of randomly distributed TiO2 nanoparticles accelerates the aging rate of the material. However, when the nanoparticles are realigned into a pillar structure, the aging rate significantly decreases. Moreover, in our experimental time scale, a dual-relaxation mechanism of aging is observed in the PMMA/TiO2 nanocomposites. This work highlights the importance of particle alignment and structure on the aging behavior of polymer nanocomposites, which could have implications for designing materials with improved stability in applications that require slow aging.The physical aging of electric field-treated PMMA-TiO2 nanocomposites is substantially reduced from its counterpart with nanoparticles randomly dispersed in the polymer host.
dc.publisherJohn Wiley & Sons, Inc.
dc.subject.othercomposites
dc.subject.otherageing
dc.subject.otherdifferential scanning calorimetry (DSC)
dc.titleSuppressed physical aging in PMMA-titanium oxide nanocomposites by controlling alignment of nanoparticles
dc.typeArticle
dc.rights.robotsIndexNoFollow
dc.subject.hlbsecondlevelChemical Engineering
dc.subject.hlbsecondlevelChemistry
dc.subject.hlbsecondlevelManagement
dc.subject.hlbtoplevelScience
dc.subject.hlbtoplevelBusiness and Economics
dc.subject.hlbtoplevelEngineering
dc.description.peerreviewedPeer Reviewed
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/177224/1/app54030.pdf
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/177224/2/app54030_am.pdf
dc.identifier.doi10.1002/app.54030
dc.identifier.sourceJournal of Applied Polymer Science
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dc.working.doiNOen
dc.owningcollnameInterdisciplinary and Peer-Reviewed


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