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CO oxidation of Pt/Al2O3 and Pd/ Al2O3 transient response and concentration cycling studies

dc.contributor.authorZhou, X.en_US
dc.contributor.authorGulari, Erdoganen_US
dc.date.accessioned2006-04-07T19:40:47Z
dc.date.available2006-04-07T19:40:47Z
dc.date.issued1986en_US
dc.identifier.citationZhou, X., Gulari, Erdogan (1986)."CO oxidation of Pt/Al2O3 and Pd/ Al2O3 transient response and concentration cycling studies." Chemical Engineering Science 41(4): 883-890. <http://hdl.handle.net/2027.42/26442>en_US
dc.identifier.urihttp://www.sciencedirect.com/science/article/B6TFK-444P7J3-MS/2/b6851cae599804f589d70173eddbfd01en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/26442
dc.description.abstractBy combining transient response experiments with forced concentration cycling, we were able to determine the reactive surface intermediates responsible for the large rate enhancements observed during periodic operation. According to the IR evidence on Pt the reactive surface species is a CO molecule adsorbed on a platinum atom sharing a chemisorbed oxygen with a neighbor. On Pd two different history dependent mechanisms were found to exist. One of these mechanisms is active only during concentration cycling and accounts for the major portion of the rate enhancement.en_US
dc.format.extent563862 bytes
dc.format.extent3118 bytes
dc.format.mimetypeapplication/pdf
dc.format.mimetypetext/plain
dc.language.isoen_US
dc.publisherElsevieren_US
dc.titleCO oxidation of Pt/Al2O3 and Pd/ Al2O3 transient response and concentration cycling studiesen_US
dc.typeArticleen_US
dc.rights.robotsIndexNoFollowen_US
dc.subject.hlbsecondlevelChemical Engineeringen_US
dc.subject.hlbtoplevelScienceen_US
dc.subject.hlbtoplevelEngineeringen_US
dc.description.peerreviewedPeer Revieweden_US
dc.contributor.affiliationumChemical Engineering Department, University of Michigan Ann Arbor, MI 48109, USAen_US
dc.contributor.affiliationumChemical Engineering Department, University of Michigan Ann Arbor, MI 48109, USAen_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/26442/1/0000530.pdfen_US
dc.identifier.doihttp://dx.doi.org/10.1016/0009-2509(86)87171-8en_US
dc.identifier.sourceChemical Engineering Scienceen_US
dc.owningcollnameInterdisciplinary and Peer-Reviewed


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