Show simple item record

Boundary effects in a surface reaction model for CO oxidation

dc.contributor.authorBrosilow, Benjamin J.en_US
dc.contributor.authorGulari, Erdoganen_US
dc.contributor.authorZiff, Robert M.en_US
dc.date.accessioned2010-05-06T22:38:28Z
dc.date.available2010-05-06T22:38:28Z
dc.date.issued1993-01-01en_US
dc.identifier.citationBrosilow, Benjamin J.; Gulari, Erdogan; Ziff, Robert M. (1993). "Boundary effects in a surface reaction model for CO oxidation." The Journal of Chemical Physics 98(1): 674-677. <http://hdl.handle.net/2027.42/70742>en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/70742
dc.description.abstractThe surface reaction model of Ziff, Gulari, and Barshad (ZGB) is investigated on finite systems with ‘‘hard’’ oxygen boundary conditions. The rate of production of CO2 is calculated as a function of y and system size. When the rate of CO adsorption y is above the first‐order transition value y2, the reactive region is found to extend into the system a distance ξ which scales as (y−y2)−0.40 when y→y2.en_US
dc.format.extent3102 bytes
dc.format.extent576971 bytes
dc.format.mimetypetext/plain
dc.format.mimetypeapplication/pdf
dc.publisherThe American Institute of Physicsen_US
dc.rights© The American Institute of Physicsen_US
dc.titleBoundary effects in a surface reaction model for CO oxidationen_US
dc.typeArticleen_US
dc.subject.hlbsecondlevelPhysicsen_US
dc.subject.hlbtoplevelScienceen_US
dc.description.peerreviewedPeer Revieweden_US
dc.contributor.affiliationumDepartment of Chemical Engineering, The University of Michigan, Ann Arbor, Michigan 48109‐2136en_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/70742/2/JCPSA6-98-1-674-1.pdf
dc.identifier.doi10.1063/1.464612en_US
dc.identifier.sourceThe Journal of Chemical Physicsen_US
dc.identifier.citedreferenceR. M. Ziff, E. Gulari, and Y. Barshad, Phys. Rev. Lett. 56, 2553 (1986).en_US
dc.identifier.citedreferenceM. Ehsasi, M. Matloch, O. Frank, J. H. Block, K. Christmann, F. S. Rys, and W. Hirschwald, J. Chem. Phys. 91, 4949 (1989).en_US
dc.identifier.citedreferenceE. V. Albano, J. Chem. Phys. 94, 1499 (1991).en_US
dc.identifier.citedreferenceJ. W. Evans and M. S. Miesch, Phys. Rev. Lett. 66, 833 (1991).en_US
dc.identifier.citedreferenceB. Yu, D. A. Browne, and P. Kleban, Phys. Rev. A 43, 1770 (1991).en_US
dc.identifier.citedreferenceJ. Mai and W. von Niessen, Phys. Rev. A 44, R6165 (1991).en_US
dc.identifier.citedreferenceA. Yu. Tretyakov and H. Takayasu, Phys. Rev. A 44, 8388 (1991).en_US
dc.identifier.citedreferenceD. ben-Avraham, S. Redner, D. B. Considine, and P. Meakin, J. Phys. A 23, L613 (1990).en_US
dc.identifier.citedreferenceM. Kolb and Y. Boudeville, J. Chem. Phys. 92, 3935 (1990).en_US
dc.identifier.citedreferenceJ. J. Luque, Phys. Rev. A 42, 3319 (1990).en_US
dc.identifier.citedreferenceM. Haruta, T. Kobayashi, H. Sano, and N. Yamada, Chem. Lett. , 405 (1987).en_US
dc.identifier.citedreferenceM. Huruta, N. Yamada, T. Kobayashi, and S. Iijima, J. Catal. 115, 301 (1989).en_US
dc.identifier.citedreferenceS. D. Gardner, G. B. Hoflund, D. R. Schryer, J. Schryer, B. T. Upchurch, and E. J. Kielin, Langmuir 7, 2135 (1991).en_US
dc.identifier.citedreferenceS. D. Gardner, G. B. Hoflund, M. R. Davidson, H. A. Laitinen, D. R. Schryer, and B. T. Upchurch, Langmuir 7, 2140 (1991).en_US
dc.identifier.citedreferenceI. Jensen, H. C. Fogedby, and R. Dickman, Phys. Rev. A 41, 3411 (1990).en_US
dc.identifier.citedreferenceG. Grinstein, Z. W. Lai, and D. A. Browne, Phys. Rev. A 40, 4820 (1989).en_US
dc.identifier.citedreferenceP. Meakin and D. J. Scalapino, J. Chem. Phys. 87, 731 (1987).en_US
dc.identifier.citedreferenceT. Engel and G. Ertyl, J. Chem. Phys. 69, 1267 (1978).en_US
dc.identifier.citedreferenceT. Engel and G. Ertyl, Adv. Catal. 28, 1 (1979).en_US
dc.identifier.citedreferenceB. C. Gates, J. R. Katzer, and G. C. A. Schuit, Chemistry of Catalytic Process (McGraw-Hill, New York, 1979).en_US
dc.identifier.citedreferenceZiff and Brosilow (to be published).en_US
dc.owningcollnamePhysics, Department of


Files in this item

Show simple item record

Remediation of Harmful Language

The University of Michigan Library aims to describe library materials in a way that respects the people and communities who create, use, and are represented in our collections. Report harmful or offensive language in catalog records, finding aids, or elsewhere in our collections anonymously through our metadata feedback form. More information at Remediation of Harmful Language.

Accessibility

If you are unable to use this file in its current format, please select the Contact Us link and we can modify it to make it more accessible to you.