Boundary effects in a surface reaction model for CO oxidation
dc.contributor.author | Brosilow, Benjamin J. | en_US |
dc.contributor.author | Gulari, Erdogan | en_US |
dc.contributor.author | Ziff, Robert M. | en_US |
dc.date.accessioned | 2010-05-06T22:38:28Z | |
dc.date.available | 2010-05-06T22:38:28Z | |
dc.date.issued | 1993-01-01 | en_US |
dc.identifier.citation | Brosilow, Benjamin J.; Gulari, Erdogan; Ziff, Robert M. (1993). "Boundary effects in a surface reaction model for CO oxidation." The Journal of Chemical Physics 98(1): 674-677. <http://hdl.handle.net/2027.42/70742> | en_US |
dc.identifier.uri | https://hdl.handle.net/2027.42/70742 | |
dc.description.abstract | The surface reaction model of Ziff, Gulari, and Barshad (ZGB) is investigated on finite systems with ‘‘hard’’ oxygen boundary conditions. The rate of production of CO2 is calculated as a function of y and system size. When the rate of CO adsorption y is above the first‐order transition value y2, the reactive region is found to extend into the system a distance ξ which scales as (y−y2)−0.40 when y→y2. | en_US |
dc.format.extent | 3102 bytes | |
dc.format.extent | 576971 bytes | |
dc.format.mimetype | text/plain | |
dc.format.mimetype | application/pdf | |
dc.publisher | The American Institute of Physics | en_US |
dc.rights | © The American Institute of Physics | en_US |
dc.title | Boundary effects in a surface reaction model for CO oxidation | en_US |
dc.type | Article | en_US |
dc.subject.hlbsecondlevel | Physics | en_US |
dc.subject.hlbtoplevel | Science | en_US |
dc.description.peerreviewed | Peer Reviewed | en_US |
dc.contributor.affiliationum | Department of Chemical Engineering, The University of Michigan, Ann Arbor, Michigan 48109‐2136 | en_US |
dc.description.bitstreamurl | http://deepblue.lib.umich.edu/bitstream/2027.42/70742/2/JCPSA6-98-1-674-1.pdf | |
dc.identifier.doi | 10.1063/1.464612 | en_US |
dc.identifier.source | The Journal of Chemical Physics | en_US |
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dc.owningcollname | Physics, Department of |
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