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Ion-beam-induced amorphization and order-disorder transition in the murataite structure

dc.contributor.authorLian, Jieen_US
dc.contributor.authorWang, L. M.en_US
dc.contributor.authorEwing, Rodney C.en_US
dc.contributor.authorYudintsev, Sergey V.en_US
dc.contributor.authorStefanovsky, Sergey V.en_US
dc.date.accessioned2011-11-15T16:04:03Z
dc.date.available2011-11-15T16:04:03Z
dc.date.issued2005-06-01en_US
dc.identifier.citationLian, Jie; Wang, L. M.; Ewing, Rodney C.; Yudintsev, Sergey V.; Stefanovsky, Sergey V. (2005). "Ion-beam-induced amorphization and order-disorder transition in the murataite structure." Journal of Applied Physics 97(11): 113536-113536-8. <http://hdl.handle.net/2027.42/87577>en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/87577
dc.description.abstractMurataite (A3B6C2O22−x/2,F3m)(A3B6C2O22−x∕2,F4¯3m), a derivative of an anion-deficient fluorite structure, has been synthesized as different polytypes as a result of cation ordering. Ion-beam-induced amorphization has been investigated by 1-MeV1-MeV Kr2+Kr2+ ion irradiation with in situ transmission electron microscopy. The critical amorphization dose was determined as a function of temperature and the degree of structural disordering. A lower critical amorphization temperature ( ∼ 860 K)(∼860K) was obtained for the disordered murataite as compared with that of the murataite superstructure (930 to 1060 K)(930to1060K). An ion-beam-induced ordered murataite to a disordered fluorite transition occurred in the murataite superstructure, similar to that observed in the closely related pyrochlore structure-type, A2B2O7A2B2O7. The ion-beam-induced defect fluorite structure is more energetically stable in the murataite structure with a higher degree of structural disordering, as compared with the murataite superstructure. This suggests that the degree of intrinsic structural disorder has a significant effect on the energetics of structural disordering process; this affects the tendency toward the order-disorder structural transition for fluorite-related compounds and their response to ion-beam-induced amorphization.en_US
dc.publisherThe American Institute of Physicsen_US
dc.rights© The American Institute of Physicsen_US
dc.titleIon-beam-induced amorphization and order-disorder transition in the murataite structureen_US
dc.typeArticleen_US
dc.subject.hlbsecondlevelPhysicsen_US
dc.subject.hlbtoplevelScienceen_US
dc.description.peerreviewedPeer Revieweden_US
dc.contributor.affiliationumDepartment of Geological Sciences, Department of Nuclear Engineering and Radiological Sciences, and Department of Materials Science and Engineering, University of Michigan, Ann Arbor, Michigan 48109en_US
dc.contributor.affiliationotherInstitute of Geology of Ore Deposits, Russian Academy of Sciences (RAS), Staromonetnii Pereulok 35, Moscow 109017, Russiaen_US
dc.contributor.affiliationotherSchneizerischer Ingenieur-und Architektenverein (SIA) Radon, 7th Rostovskii Pereulok 2/14, Moscow 119121, Russiaen_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/87577/2/113536_1.pdf
dc.identifier.doi10.1063/1.1926394en_US
dc.identifier.sourceJournal of Applied Physicsen_US
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dc.owningcollnamePhysics, Department of


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