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Spectral phase effects on nonlinear resonant photochemistry of 1,3-cyclohexadiene in solution
dc.contributor.authorCarroll, E. C.en_US
dc.contributor.authorPearson, B. J.en_US
dc.contributor.authorFlorean, Andrei C.en_US
dc.contributor.authorBucksbaum, Philip H.en_US
dc.contributor.authorSension, Roseanne J.en_US
dc.date.accessioned2011-11-15T16:10:34Z
dc.date.available2011-11-15T16:10:34Z
dc.date.issued2006-03-21en_US
dc.identifier.citationCarroll, E. C.; Pearson, B. J.; Florean, A. C.; Bucksbaum, P. H.; Sension, Roseanne J. (2006). "Spectral phase effects on nonlinear resonant photochemistry of 1,3-cyclohexadiene in solution." The Journal of Chemical Physics 124(11): 114506-114506-10. <http://hdl.handle.net/2027.42/87876>en_US
dc.identifier.urihttps://hdl.handle.net/2027.42/87876
dc.description.abstractWe have investigated the ring opening of 1,3-cyclohexadiene to form 1,3,5-cis-hexatriene (Z-HT) using optical pulse shaping to enhance multiphoton excitation. A closed-loop learning algorithm was used to search for an optimal spectral phase function, with the effectiveness or fitness of each optical pulse assessed using the UV absorption spectrum. The learning algorithm was able to identify pulses that increased the formation of Z-HT by as much as a factor of 2 and to identify pulse shapes that decreased solvent fragmentation while leaving the formation of Z-HT essentially unaffected. The highest yields of Z-HT did not occur for the highest peak intensity laser pulses. Rather, negative quadratic phase was identified as an important control parameter in the formation of Z-HT.en_US
dc.publisherThe American Institute of Physicsen_US
dc.rights© The American Institute of Physicsen_US
dc.titleSpectral phase effects on nonlinear resonant photochemistry of 1,3-cyclohexadiene in solutionen_US
dc.typeArticleen_US
dc.subject.hlbsecondlevelPhysicsen_US
dc.subject.hlbtoplevelScienceen_US
dc.description.peerreviewedPeer Revieweden_US
dc.contributor.affiliationumFOCUS Center, University of Michigan, 500 East University Avenue, Ann Arbor, Michigan 48109-1120en_US
dc.identifier.pmid16555900en_US
dc.description.bitstreamurlhttp://deepblue.lib.umich.edu/bitstream/2027.42/87876/2/114506_1.pdf
dc.identifier.doi10.1063/1.2168454en_US
dc.identifier.sourceThe Journal of Chemical Physicsen_US
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dc.owningcollnamePhysics, Department of


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