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- Creator:
- Ye, Zhengwei and Mi, Zetian
- Description:
- Generation of C2+ compounds using sunlight, carbon dioxide, and water provides a promising path for carbon neutrality. The exploration of a catalyst to break the bottleneck of C-C coupling, for constructing a rational artificial photosynthesis integrated device, is at the core. Herein, based on operando spectroscopy measurements, theoretical calculations, and feedstock experiments, it is discovered that gold, in conjunction with iridium, can catalyze the reduction of CO2, achieving C-C coupling by insertion of CO2 into -CH3. Owing to a combination of optoelectronic and catalytic properties, the assembly of AuIr with InGaN nanowires on silicon (AuIr@InGaN NWs/Si) enables the achievement of a C2H6 activity of 58.8 mmol‧g-1‧h-1 with a turnover number of 54,595 over 60 hours. A light-to-fuels efficiency of ~0.59% for solar fuels production from CO2 and H2O is achieved without any other energy inputs. This work provides a carbon-negative path for producing higher order C compounds.
- Keyword:
- Carbon dioxide reduction and Photocatalysis
- Discipline:
- Science
-
- Creator:
- Martin, Tara L, Young, LR, Goldsteen, D, Nunamaker, EA, Reynolds, P, Thompson-Iritani, S, Thurston, SE, and LaFollette, MR
- Description:
- This dataset contains the results of a survey of mouse handling methods by personnel working with laboratory mice. The survey included questions about preferred handling methods, barriers to use of refined handling methods, and a knowledge quiz about refined mouse handling. Data was collected via Qualtrics survey as described in the methodology section. This dataset is associated with the following publication, accepted by PLOS One: PONE-D-23-01633R1 Title: Using refined methods to pick up mice: A survey benchmarking prevalence & beliefs about tunnel and cup handling Authors: Lauren Young, Donna Goldsteen, Elizabeth A. Nunamaker, Mark J. Prescott, Penny Reynolds, Sally Thompson-Iritani, Sarah E. Thurston, Tara L. Martin, Megan R. LaFollette
- Keyword:
- Mouse, Refined Handling, Tunnel Handling, Cup Handling, Laboratory Animal, and Animal Care
- Citation to related publication:
- Young LR, Goldsteen D, Nunamaker EA, Prescott MJ, Reynolds P, Thompson-Iritani S, Thurston SE, Martin TL, LaFollette MR. Using refined methods to pick up mice: A survey benchmarking prevalence & beliefs about tunnel and cup handling. PLOS ONE. 2023. In Press.
- Discipline:
- Science
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- Creator:
- Dewey, Ryan M, Livi, Stefano, Lepri, Susan T, Raines, Jim M, Ploof, Keeling, and The HIS Science Team
- Description:
- The data contained within the archive are for analysis and replication of Figure 2 in Livi et al. (2023), First Results from the Solar Orbiter Heavy Ion Sensor, Astronomy & Astrophysics. The readme.txt file contains more details on the contents of the archive and its files. Livi et al. (2023) reports the first solar wind composition measurements collected from the Heavy Ion Sensor (HIS) on the Solar Orbiter spacecraft. The period of study spans January-June 2022 during with the spacecraft completed nearly a full orbit about the Sun, from 0.3 AU to 1.0 AU. The solar wind composition within this publication are the first within the inner heliosphere. This paper describes the data and its processing from raw measurements (e.g., the data contained within this archive) to derived composition data products, and examines these composition data products about an interplanetary shock and interplanetary coronal mass ejection. Finally, these composition data are examined statistically and compared to historical data sets.
- Keyword:
- Solar Orbiter, Solar wind, Heavy ions, and Heavy Ion Sensor
- Citation to related publication:
- Livi, S., et al. (2023), First Results from the Solar Orbiter Heavy Ion Sensor, Astronomy & Astrophysics. https://doi.org/10.1051/0004-6361/202346304 and Owen, C., et al. (2020), The Solar Orbiter Solar Wind Analyser (SWA) suite, Astronomy & Astrophysics, 642. https://doi.org/10.1051/0004-6361/201937259
- Discipline:
- Science
-
- Creator:
- Thompson, Ellen P. and Ellis, Brian R.
- Description:
- Accurate prediction of physical alterations in carbonate reservoirs under dissolution is critical for development of subsurface energy technologies. The impact of mineral dissolution on flow characteristics depends on the connectivity and tortuosity of the pore network. Persistent homology is a tool from algebraic topology that describes the size and connectivity of topological features. When applied to 3D X-ray computed tomography (XCT) imagery of rock cores, it provides a novel metric of pore network heterogeneity. Prior works have demonstrated the efficacy of persistent homology in predicting flow properties in numerical simulations of flow through porous media. Its ability to combine size, spatial distribution, and connectivity information make it a promising tool for understanding reactive transport in complex pore networks, yet limited work has been done to apply persistence analysis to experimental studies on natural rocks. In this study, three limestone cores were imaged by XCT before and after acid-driven dissolution flow through experiments. Each XCT scan was analyzed using persistent homology. In all three rocks, permeability increase was driven by the growth of large, connected pore bodies. The two most homogenous samples saw an increased effect nearer to the flow inlet, suggesting emerging preferential flow paths as the reaction front progresses. The most heterogeneous sample showed an increase in along-core homogeneity during reaction. Variability of persistence showed moderate positive correlation with pore body size increase. Persistence heterogeneity analysis could be used to anticipate where greatest pore size evolution may occur in a reservoir targeted for subsurface development, improving confidence in project viability.
- Keyword:
- Carbonate dissolution, X-ray computed tomography, Porous media, Topology, and Persistent homology
- Citation to related publication:
- Thompson, E.P.; Ellis, B.R. (2023) Persistent Homology as a Heterogeneity Metric for Predicting Pore Size Change in Dissolving Carbonates. In Review.
- Discipline:
- Science and Engineering
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- Creator:
- Bellile, Emily L, Taylor, Jeremy MG, and Wolf, Gregory T
- Description:
- The University of Michigan’s Head and Neck Specialized Program of Research Excellence (SPORE) included an epidemiology project that approached every previously untreated adult head and neck squamous carcinoma (HNSCC) patient evaluated in the multidisciplinary Head and Neck Oncology Program of the University of Michigan (UM; Ann Arbor, MI) Comprehensive Cancer Center for participation in our longitudinal epidemiology study. This analytic dataset includes the most commonly requested covariates and outcome variables for survival analysis of this cohort of HNSCC patients. Data cleaning and creation of this analysis dataset was performed with SAS software v 9.3 (Carey,NC) by a biostatistician supporting multiple projects in the University of Michigan’s Head and Neck Specialized Program of Research Excellence (SPORE) and is available in RedCap for UM investigators to join with discipline specific data collected on the same cohort through a de-identified ID link.
- Keyword:
- Head and Neck Cancer, HNSCC, Squamous Cell Cancer, Epidemiology, Head and Neck Specialized Program of Research Excellence (SPORE). , Cancer, Prognosis, and Survival Analysis
- Citation to related publication:
- Cigarette use, comorbidities, and prognosis in a prospective head and neck squamous cell carcinoma population. Peterson LA, Bellile EL, Wolf GT, Virani S, Shuman AG, Taylor JM, Rozek LS; University of Michigan Head and Neck Specialized Program of Research Excellence Program. Head Neck. 2016 Dec;38(12):1810-1820. doi: 10.1002/hed.24515. Epub 2016 Jul 19. PMID: 27432208. , Development and Assessment of a Model for Predicting Individualized Outcomes in Patients With Oropharyngeal Cancer. Beesley LJ, Shuman AG, Mierzwa ML, Bellile EL, Rosen BS, Casper KA, Ibrahim M, Dermody SM, Wolf GT, Chinn SB, Spector ME, Baatenburg de Jong RJ, Dronkers EAC, Taylor JMG. JAMA Netw Open. 2021 Aug 2;4(8):e2120055. doi: 10.1001/jamanetworkopen.2021.20055. PMID: 34369988., Amlani, L; Bellile, E; Spector, M; Smith, J; Brenner, C; Rozek, L; Nguyen, A; Zarins, K; Thomas, D; McHugh, J; Taylor, J; Wolf, GT. Expression of p53 and prognosis in patients with head and neck squamous cell carcinoma (HNSCC); Int J Cancer Clin Res 2019, 6:122. DOI: 10.23937/2378-3419/1410122., and Spector ME, Bellile E, Amlani L, Zarins K, Smith J, Brenner JC, Rozek L, Nguyen A, Thomas D, McHugh JB, Taylor JMG, Wolf GT; University of Michigan Head and Neck SPORE Program. Prognostic Value of Tumor-Infiltrating Lymphocytes in Head and Neck Squamous Cell Carcinoma. JAMA Otolaryngol Head Neck Surg. 2019 Nov 1;145(11):1012-1019. doi: 10.1001/jamaoto.2019.2427. PMID: 31486841; PMCID: PMC6735419.
- Discipline:
- Science and Health Sciences
-
- Creator:
- University of Michigan Museum of Paleontology and CTEES
- Description:
- Reconstructed CT slices for navicular of Cantius trigonodus (University of Michigan Museum of Paleontology catalog number UMMP 87973) as a series of TIFF images. Raw projections are not included in this dataset. The reconstructed slice data from the scan are offered here as a series of unsigned 16-bit integer TIFF images. The upper left corner of the first image (*_0000.tif) is the XYZ origin.
- Keyword:
- Paleontology, Fossil, CT, Notharctidae, UMMP, University of Michigan Museum of Paleontology, Eocene, and a537f0d8-6185-9562-9b9a-a233468bf8e1
- Discipline:
- Science
-
- Creator:
- University of Michigan Museum of Paleontology and CTEES
- Description:
- Reconstructed CT slices for L cuboid of Cantius mckennai (University of Michigan Museum of Paleontology catalog number UMMP 81824) as a series of TIFF images. Raw projections are not included in this dataset. The reconstructed slice data from the scan are offered here as a series of unsigned 16-bit integer TIFF images. The upper left corner of the first image (*_0000.tif) is the XYZ origin.
- Keyword:
- Paleontology, Fossil, CT, Notharctidae, UMMP, University of Michigan Museum of Paleontology, Eocene, and e763ae30-4a86-9d02-0b8a-9297ff48cf58
- Discipline:
- Science
-
- Creator:
- University of Michigan Museum of Paleontology and CTEES
- Description:
- Reconstructed CT slices for navicular of Cantius trigonodus (University of Michigan Museum of Paleontology catalog number UMMP 73318) as a series of TIFF images. Raw projections are not included in this dataset. The reconstructed slice data from the scan are offered here as a series of unsigned 16-bit integer TIFF images. The upper left corner of the first image (*_0000.tif) is the XYZ origin.
- Keyword:
- Paleontology, Fossil, CT, Notharctidae, Eocene, and 0d607d85-8d27-6be2-dbc5-9cb73f1324ae
- Discipline:
- Science
-
- Creator:
- Zhang, Yingxiao MI and Steiner, Allison MI
- Description:
- Atmospheric aerosols are emitted from both natural and anthropogenic sources, and they play an important role in climate, impacting solar radiation and cloud formation. Compared to other types of aerosol particles, primary biological aerosol particles (PBAP, e.g., fungal spores, bacteria, pollen, virus, etc.) are relatively understudied. However, they are linked to adverse health effects and have the potential to influence ice nucleation at higher temperatures. Anemophilous (or wind-driven) pollen is one of the important PBAP, impacts cloud properties under some conditions, and triggers allergic diseases such as allergic rhinitis (also known as hay fever) and asthma. Because pollen emission is closely associated with environmental drivers, the climatic change could influence pollen emission and consequently the incidence of allergic disease. Using CMIP6 model data, our research projects continental-scale changes in pollen emissions at the end of the century, considering the effects of temperature, precipitation, CO2, and future vegetation distribution change. While prior studies have evaluated single types of pollen, we use a mechanistic model to comprehensively simulate total pollen across the United States from all sources. Similar to previous single-source pollen studies, our simulations suggest that pollen season duration will lengthen, and pollen emission will increase in the future, but in addition, we identify new synergies between different pollen types that can influence the maximum daily pollen. Our work highlights that the changes of overlap between pollen seasons of different vegetation taxa can magnify or mitigate the impacts of climate change, which addresses the importance to study all pollen emissions comprehensively. Given pollen is one of the most common triggers of seasonal allergies, our findings also provide information to evaluate global health conditions in the future. In this study, all of the pollen emission data are written in NetCDF files.
- Keyword:
- Pollen emission change, Climate change, Public health, Vegetation land cover change, and CO2 effects
- Citation to related publication:
- Zhang, Y. and Steiner, A. “Projected climate-driven changes in pollen emission season length and magnitude over the continental United States”, under review in Nature Communication, 2022. and yingxz. (2022). steiner-lab/pecm: PECM2.0 (2.0). Zenodo. https://doi.org/10.5281/zenodo.5874177
- Discipline:
- Science
-
- Creator:
- Bradshaw, Lisa, Vernon, Julianne, Schmidt, Thomas, James, Timothy, Zhang, Jianzhi, Archbold, Hilary, Cadigan, Ken, Wolfe, John P., and Goldberg, Deborah E.
- Description:
- This is the experimental data referenced in our manuscript entitled "Influence of CUREs on STEM retention depends on demographic identities." The dataset comprises csv files with results from student surveys given to students enrolled in Biology 173 from Fall 2015 through Fall 2019 as well as institutional data of their course grades and cumulative GPA at the time they enrolled in Biology 173, and graduation and major data for student who had graduated by 2021. The survey questions used in the analysis and the IRB consent form are also included as pdfs.
- Keyword:
- undergraduate research, STEM retention, CURE, introductory biology laboratory, and education research
- Citation to related publication:
- Bradshaw, L., Vernon J., Schmidt T., James T., Zhang J., Archbold H., Cadigan K., Wolfe J.P. & Goldberg D. 2023. Research article: Influence of CUREs on STEM retention depends on demographic identities. J Microbiol Biol Educ (accepted)
- Discipline:
- Science